- Outfielder for the St. Louis Cardinals
- He is a nine-time winner of the James "Tip" O'Neill Award, presented annually by the Canadian Baseball Hall of Fame & Museum (individual achievement while adhering to the highest ideals of baseball).
- He was playing baseball for the Canadian National Junior Team when Expos scouts discovered him, he originally grew up a hockey goaltender, playing for 13 years, and teaming with former Bruins all-star Cam Neely before pursuing a baseball career
- Signed with the Colorado Rockies in 1995
- Larry and his wife, Angela have two daughters Canaan Rose-Lynn (b. 2001) and Shayna Kaitlin (b. 2003) and he has another daughter Brittany Marie (b. 1995) from a previous relationship
- Is the Colorado Rockies all-time leader in many categories
- Outfielder with the National League's Montreal Expos (1989-1994), Colorado Rockies (1995-2003), and St. Louis Cardinals (2004).
- Made major league debut on 16 August 1989.
- Named to Baseball Digest magazine's 1990 Rookie All-Star Team.
- When living in the Denver area, he was a season ticket holder of the Colorado Avalanche of the National Hockey League
- Once listed on the Western Hockey League's Regina Pats 50 man "protected" list, around 1985, as a goaltender.
- Once said that if he could be a goaltender in the National Hockey League and have all the skills for it, he would leave baseball immediately (Walker's first love).
- Voted into the National Baseball Hall of Fame in 2020. The 2020 induction ceremony was canceled because of the COVID-19 pandemic, and he was inducted in 2021, along with members of that year's class.
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